Formation of perfect ohmic contact at indium tin oxide/N,N'-di(naphthalene-1-yl)-N,N'-diphenyl-benzidine interface using ReO3.
Identifieur interne : 000177 ( Main/Exploration ); précédent : 000176; suivant : 000178Formation of perfect ohmic contact at indium tin oxide/N,N'-di(naphthalene-1-yl)-N,N'-diphenyl-benzidine interface using ReO3.
Auteurs : RBID : pubmed:24469505Abstract
A perfect ohmic contact is formed at the interface of indium tin oxide (ITO) and N,N'-di(naphthalene-1-yl)-N,N'-diphenyl-benzidine (NPB) using ReO3 as the interfacial layer. The hole injection efficiency is close to 100% at the interface, which is much higher than those for interfacial layers of 1,4,5,8,9,11-hexaazatripheylene hexacarbonitrile (HAT-CN) and MoO3. Interestingly, the ReO3 and MoO3 interfacial layers result in the same hole injection barrier, ≈0.4 eV, to NPB, indicating that the Fermi level is pinned to the NPB polaron energy level. However, a significant difference is observed in the generated charge density in the NPB layer near the interfacial layer/NPB interface, indicating that charge generation at the interface plays an important role in forming the ohmic contact.
DOI: 10.1038/srep03902
PubMed: 24469505
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<author><name sortKey="Yoo, Seung Jun" uniqKey="Yoo S">Seung-Jun Yoo</name>
<affiliation wicri:level="1"><nlm:affiliation>WCU Hybrid Materials Program, Department of Materials Science and Engineering and the Center for Organic Light-Emitting Diodes, Seoul National University, Seoul 151-744, South Korea.</nlm:affiliation>
<country xml:lang="fr">Corée du Sud</country>
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<author><name sortKey="Chang, Jung Hung" uniqKey="Chang J">Jung-Hung Chang</name>
<affiliation wicri:level="1"><nlm:affiliation>Graduated Institute of Photonics and Optoelectronics and Department of Electrical Engineering, National Taiwan University, Taipei 106, Taiwan.</nlm:affiliation>
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<wicri:regionArea>Graduated Institute of Photonics and Optoelectronics and Department of Electrical Engineering, National Taiwan University, Taipei 106</wicri:regionArea>
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<author><name sortKey="Lee, Jeong Hwan" uniqKey="Lee J">Jeong-Hwan Lee</name>
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<author><name sortKey="Moon, Chang Ki" uniqKey="Moon C">Chang-Ki Moon</name>
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<author><name sortKey="Wu, Chih I" uniqKey="Wu C">Chih-I Wu</name>
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<author><name sortKey="Kim, Jang Joo" uniqKey="Kim J">Jang-Joo Kim</name>
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<front><div type="abstract" xml:lang="en">A perfect ohmic contact is formed at the interface of indium tin oxide (ITO) and N,N'-di(naphthalene-1-yl)-N,N'-diphenyl-benzidine (NPB) using ReO3 as the interfacial layer. The hole injection efficiency is close to 100% at the interface, which is much higher than those for interfacial layers of 1,4,5,8,9,11-hexaazatripheylene hexacarbonitrile (HAT-CN) and MoO3. Interestingly, the ReO3 and MoO3 interfacial layers result in the same hole injection barrier, ≈0.4 eV, to NPB, indicating that the Fermi level is pinned to the NPB polaron energy level. However, a significant difference is observed in the generated charge density in the NPB layer near the interfacial layer/NPB interface, indicating that charge generation at the interface plays an important role in forming the ohmic contact.</div>
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<Abstract><AbstractText>A perfect ohmic contact is formed at the interface of indium tin oxide (ITO) and N,N'-di(naphthalene-1-yl)-N,N'-diphenyl-benzidine (NPB) using ReO3 as the interfacial layer. The hole injection efficiency is close to 100% at the interface, which is much higher than those for interfacial layers of 1,4,5,8,9,11-hexaazatripheylene hexacarbonitrile (HAT-CN) and MoO3. Interestingly, the ReO3 and MoO3 interfacial layers result in the same hole injection barrier, ≈0.4 eV, to NPB, indicating that the Fermi level is pinned to the NPB polaron energy level. However, a significant difference is observed in the generated charge density in the NPB layer near the interfacial layer/NPB interface, indicating that charge generation at the interface plays an important role in forming the ohmic contact.</AbstractText>
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